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BRIEF RESEARCH REPORT article

Front. Phys., 05 August 2024
Sec. Fusion Plasma Physics
This article is part of the Research Topic Proton Boron Nuclear Fusion: From Energy Production to Medical Applications View all 7 articles

On the ignition of H11B fusion fuel

  • 1HB11 Energy Holdings Ltd Pty, Sydney, NSW, Australia
  • 2School of Electrical Engineering and Telecommunications, Faculty of Engineering, UNSW Sydney, Kensington, NSW, Australia

We have revisited recent results on the ideal ignition of H11B fuel, in the light of the latest available reactivity, an alternative self-consistent calculation of the electron temperature, an increased extent of the suprathermal effects and the impact of plasma density. At high density, we find that the ideal ignition temperature is appreciably relaxed (e.g., Ti150 keV for ni1026cm3 and an optimal 11B/H concentration ε=0.15) and burn becomes substantial. We have then investigated central hot-spot ignition in both isobaric and isochoric inertial confinement configurations. Although implosion-driven ignition appears to be unfeasible, the isochoric self-heating conditions foster favourable preliminary conclusions on the utilization of proton fast ignition. In the isochoric case, we find a broad minimum in the ignition energy at ρR8.5g/cm2 and 220Ti340 keV (80 Te95 keV), for ε=0.15.

1 Introduction

The 11B(p,3α) fusion reaction, with a Q-value of 8.6 MeV, is experiencing a renewed interest for energy production purposes, in the light of recent experimental and theoretical findings [111]. The reaction is aneutronic and involves only abundant and stable isotopes. Moreover, the α particles in its final state may release all their energy to the fusion plasma. The reaction is also of interest for studies in stellar evolution, where relative abundances of 11B, Li and Be provide insight into stellar processes [12]. Proposed approaches for energy production span magnetic [13], magneto-inertial [14, 15] and laser-driven [5, 16, 17] fusion. The exploitation of H11B fuel, however, remains extremely challenging because of its low reactivity and high radiative losses at temperatures attainable in present-day fusion devices.

The existence of ideal ignition conditions has been demonstrated only lately by Putvinski et al. [6], who have used a recent fusion cross section dataset [4] for the calculation of the thermal reactivity and added to this latter a contribution coming from kinetic (particularly, suprathermal) effects, calculated self-consistently. Suprathermal effects are due to elastic collisions between the fusion-born α′s and background thermal protons [6, 18], which develop a bolder tail in the proton energy spectrum compared to the Maxwell-Boltzmann distribution [1921]. Putvinski et al. [6] have found fusion power to overcome bremsstrahlung losses only marginally, for 250Ti380 keV, in a dilute plasma (ni=np+nB= 1014 cm-3) at the optimal 11B/H ion concentration εnB/np=0.15, with Te calculated self-consistently (standard notation is used).

In this Brief Research Report, we first revisit those findings in the light of the latest available reactivity, an alternative self-consistent calculation of Te as well as the actual extent of the suprathermal effects. We then show how ideal ignition conditions vary depending on the plasma density regime, the extent of suprathermal effects and the boron-to-hydrogen concentration. We find a relaxed ignition temperature and a significantly larger fusion-to-bremsstrahlung power ratio at high density. Consequently, we study ignition in actual isobaric and isochoric hot-spot fuel configurations, and draw preliminary conclusions on fast ignition.

We recall that hot-spot fuel configurations are relevant to laser-driven inertial confinement, which is a promising method to achieve fusion energy [22]. Ignition of DT fuel has recently been achieved at the US National Ignition Facility [23], by exploiting an indirect-drive scheme based on a nearly isobaric fuel configuration [24]. Fast ignition is a technique alternative to hot-spot ignition and is based on the ignition of precompressed fuel by means of an external trigger. Laser-driven fast ignition was proposed by Tabak et al. [25] 30 years ago and it is today the subject of significant theoretical and experimental investigation [26, 27].

2 Ideal ignition

The ideal ignition conditions of Putvinski et al. [6] have been recalculated and plotted in Figure 1A (blue curve) in terms of the ratio Pf/Pb, where

PfTi=1+sPthTi(1)

is the fusion power (per unit volume), Pth is the thermal fusion power, s is a parameter expressing the suprathermal contribution, and PbTe is the bremsstrahlung power (see Appendix A for formulas). While s=0.1 has been found by Putvinski et al., large-angle scattering, particularly by the effect of the nuclear (strong) interaction, does not appear to have been taken into account in their α-p collision calculations. One of us has shown [20] that in a H11B plasma at high density (ne∼1026 cm-3) and electron temperature (Te50 keV), suprathermal effects calculated on the basis of the complete elastic α-p cross section can be approximately two times higher than those found upon the assumption of a pure Coulomb scattering. Accordingly, we put forward that s is very likely to reach 0.2. This assumption is in line with the earliest findings of Weaver et al. [19], who calculated a suprathermal increase of the H11B reaction rate up to 15% at high plasma density and temperature, based on kinetic simulations that included both Coulomb and nuclear large-angle scattering (but that were biased by the poor knowledge of the relevant elastic and fusion cross sections at that time).

Figure 1
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Figure 1. (A) Revisit of Putvinski et al’s ideal ignition and burn conditions [6], at low plasma density. (B) TeTi characteristic curves, calculated self-consistently at low and high plasma density (s=0.1). (C, D) High-density case: Pf/Pb vs. Ti and ideal ignition temperature at low and high 11B concentration (ε=0.15,0.5), for representative values of s.

From Figure 1A, we note that ignition is not possible if the suprathermal contribution is not accounted for (s=0, black curve). We also note that the region where Pf/Pb1 extends to higher values of Ti (up to 440 keV) compared to Ref. [6], which is very likely due to the fact that we have used a more accurate (and appreciably higher) reactivity [28] in the calculation of Pth.

As for the self-consistent calculation of Te, we recall that in the TiTe plane of an ideal plasma, the self-burn region is bounded by the solutions of the steady-state power balance equations (29)

PfPb=0(2)
ηiPfPie=0(3)

where ηi is the fraction of the fusion power transferred to the ions by the α particles and Pie is the power transferred from the ions to the electrons (see Appendix A). Eq. 2 is the balance equation for the entire system and gives the maximum possible Te, Te,max, at any Ti higher than the ideal ignition temperature, Tid, while Eq. 3 holds for the ion fluid only and gives the minimum possible Te, Te,min (Figure 1B). All the possible trajectories of the system during burn, which are determined by the time-dependent power flow equations (and their initial conditions) for the ion and electron fluids, lie between the Te,min and Te,max curves. We have used Eq. 3 to obtain the TeTi relationship (blue curve in Figure 1B), whereas Putvinski et al. have used the power balance equation for the electron fluid, i.e.,

1ηiPf+PiePb=0(4)

which yields slightly higher values of Te. Those result in a lower Pf/Pb ratio compared to Figure 1A as Pb increases with Te.

While ignition and self-burn appear less marginal than previously found, low-density plasmas remain of a primary interest for magnetic confinement approaches, which can operate at sub-ignition. More meaningful conclusions can be drawn for ignition-based schemes, at high density. While the explicit square-density dependence of the P-terms cancels out in Eqs 2, 3, a residual dependence on density remains in Eq. 3 through the Coulomb logarithms of Pie −cp. Eqs A3, A4. Typical values of lnΛie at Te=100 keV are: lnΛpe24, lnΛBe22 for ne=1014cm3, and lnΛpe8,lnΛBe6 for ne=1026cm3. The change of the Coulomb logarithms upon density causes the Te,min curve in Figure 1B to shift downward while moving from a dilute to a dense plasma. As a consequence, Tid decreases and the self-burn region enlarges. At high density, ignition and burn are quite substantial for H11B fuel. Note that this effect is amplified by the strong decoupling between Te and Ti, without which Pie0.

As Pb is minimum, throughout the burn region, along Te=Te,minTi, this latter condition also yields the maximum Pf/Pb ratio attainable at a given Ti. This has been plotted in Figure 1C for ni=1026cm3 (corresponding to a mass density ρ250g/cm3 for ε=0.15) and representative values of s. For s = 0.2, Tid lowers to about 150 keV, while Pf/Pb overcomes 2. Moving to ni=1027cm3 does not change Te,minTi substantially and decreases Tid only by a few keV. On another note, Te,min and Te,max are mildly sensitive to s, for s1. For instance, it is easy to see that Te,max scales approximately as 1+s2.

The high Pf/Pb ratio of Figure 1C encourages the analysis of ignition conditions in hot-spot configurations, where additional loss terms come into play, and shows the potential to withstand fuel depletion and bremsstrahlung emission due to the α-particle ash [30, 31]. It also opens the possibility of working at increased 11B concentration. Figure 1D shows Pf/Pb curves for the case of ε= 0.5. Ideal ignition can still be achieved, however subject to the suprathermal contribution and at the expenses of higher values of Tid. Ignition at equimolarity, i.e., ε=1, is confirmed to be impossible, at least for s0.2.

3 Hot-spot ignition

The power balance condition for a hot spot of radius R and density ρ at the ignition threshold reads

PfPbPhPm=0(5)

where Ph is the power density lost through heat conduction and Pm that lost through mechanical work (Pm=0 in the isobaric case); see Appendix A. All fusion born α′s are assumed to remain inside the hot spot. Eq. 5 results in a quadratic equation for ρR which coefficients, in general, are functions of Ti and Te, and depend on ε and s. Eq. 5 is coupled to either of the power balance equations for ions and electrons −analogue to Eqs. 3, 4 for the ideal case− through which the variable Te can be eliminated. It is convenient to work with the power flow equation for the ion fluid, i.e.,

ηiPfPiePm,i=0(6)

where Pm,i is the component of Pm exerted by the ions. In the isobaric case, the fact that Pm,i=0 enables the use of the same characteristic curve given by Eq. 3, in blue in Figure 1B. This self-consistent relationship can be retained also in the isochoric case, inasmuch as Pm,iPie. The isochoric ignition boundary has been generated upon this assumption (Figure 2). As a term of reference, the contour corresponding to Pm,i/Pie=0.3 has also been plotted, which shows that the condition Pm,iPie is reasonably consistent with the large ρR values entailed by the isochoric curve, due to the ρR1 dependency of Pm,i.

Figure 2
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Figure 2. Left-hand ordinate: Confinement parameter vs. Ti for self-heating of isobaric and isochoric H11B fuel assemblies. Right-hand ordinate: ρ2-weighed ignition energy for the isochoric configuration. Calculations are made for ni=1026/cm3, ε=0.15 and s=0.2.

By analogy with the DT and DD cases, we expect that 1D simulations of pre-assembled fuel would actually show a lower branch of the ignition curves in the proximity of and after their knee, due to a cooling/re-heating mechanism of the hot spot for initial points located just below the analytic curves [3235]. In the case of isochoric DT, for instance, ρR reduces by a factor of 1.5 when Ti is twice the minimum of the analytic curve, and the gap increases with Ti [35]. The difference is even more dramatic in the case of isobaric DT [3335].

Although the confinement parameter is high at the minimum of ignition curves, we have checked that the plasma is still optically thin, i.e., the Planck mean free path, lP, is much larger than R. This is due to the high electron temperature. Indeed, one has lP=ρκp1, where

κp=0.43<Z><Z2>/<A>2ρTe7/2cm2/g(7)

is the free-free Planck mean opacity [35], with

X=npXp+nBXBni=Xp+εXB1+ε(8)

For instance, ρlP9000g/cm2 at Ti=200 keV (Te=80 keV), ρ=1000g/cm3 and ε=0.15.

The ignition energy, Eig, has been calculated as the internal (thermal) energy of the hot spot in the ideal gas approximation, i.e.,

Eig=32pV=2πΓiTi+ΓeTeρR3ρ2(9)

where V is the volume of the plasma sphere and p is its pressure, as given by

p=pi+pe(10)
pie=ΓieρTie(11)
Γi=k/Amp,Γe=ZΓi(12)

The quantity ρ2Eig has been plotted vs. Ti in Figure 2 only for the isochoric case, which is expected to enable the higher gain. The curve shows a broad minimum for 220Ti340 keV, which corresponds to ρR8.5 g/cm2. One can estimate that at ρ as high as 4,000 g/cm3, Eig at its minimum is still considerably large (∼3 MJ).

4 Discussion and conclusion

Despite the fact that self-heating is possible in a pre-formed hot spot, we have verified that implosion-driven formation of the hot spot is hydrodynamically impossible, on the basis of the same argument preventing it in pure D fuel [34], i.e., a cooling timescale shorter than the hot-spot confinement time tcR/cs, being cs the isothermal sound velocity. Even without this issue, considerations on the required implosion velocity and hydrodynamic instabilities would prevent this scheme from being viable. These circumstances point toward fast ignition as possibly the only scheme to ignite inertially confined H11B fuel, apart from the trivial, low-gain case of volume ignition. Nevertheless, isochoric self-heating conditions provide a preliminary estimate of fast ignition requirements [35].

Proton fast ignition [36] is particularly suited to H11B fuel, not only because of its superior ballistic properties in the energy deposition and the potential capability of inducing the hot-ion mode, but also because of the additional heating provided by the in-flight fusion reactions of the proton beam [21, 37]. It has been put forward [21] that in a fully degenerate 11B plasma, under certain conditions, this contribution could become as large as the initial kinetic energy of the proton beam. Such an effect could then appreciably reduce the ignitor energy required in a H11B mixture. Taking also into account the reduction of Eig because of the abovementioned lowering of the higher-Ti branch of the isochoric curve −note that Eig scales as ρR3 − ignitor energies of a few hundreds kJ can be expected at densities around 4000g/cm3. The laser energy required to drive the implosion is estimated at about 1.3 MJ per mg of fuel, by assuming an overall laser-target coupling efficiency of 15% (direct drive), a unit isentrope parameter, and ε=0.15.

The ignitor pulse will have to be delivered to the compressed target within a timescale shorter than tc; e.g., tc6 ps for Ti=220 keV (Te=85 keV), ρR=10 g/cm2 and ρ = 4,000 g/cm3. Due to the progressive heating induced, the protons in the bunch will experience rapidly and drastically changing plasma conditions upon their arrival onto the hot spot, and even during their slowing down [38]. Plasma degeneracy will shift from strong at the onset of the ignitor pulse to very weak on its tail. Matching the proton range to the hot spot confinement parameter along the evolving plasma conditions will require a suitably tailored proton spectrum. The determination of such spectrum can only be carried out upon a self-consistent approach to the ignitor-fuel interaction, through accurate simulations. While this task is beyond the scope of the present study, here we estimate, for instance, that 2.5 MeV protons have a 10 g/cm2 range at the ignition conditions which have been used to calculate tc and which correspond to the last stage of the hot-spot heating process (see Appendix A for details on the stopping power). At the early stage of hot-spot heating, for e.g., Ti=Te=10 keV, the 10 g/cm2 range corresponds to a much higher proton energy, about 200 MeV. In practice, protons with a mean energy of a few tens MeV will most probably be needed. Assuming a 300 kJ ignitor, an overall number of protons of the order of 1016–1017 is estimated accordingly. As a term of comparison, a highly directional beam of 1013 protons with an approximately Maxwellian spectrum at an effective temperature of 6 MeV has been produced under intense laser irradiation (600 J, 0.5 ps, 3 × 1020 W/cm2) of thin foils, through the Target Normal Sheath Acceleration (TNSA) mechanism [39]. Driving a TNSA-based proton ignitor for H11B fuel will therefore require a multiple-beam laser firing scheme and a suitably engineered foil target (e.g., multi-spot designed, heavily H-loaded, convex-shaped for focusing the ignitor beam). The placement of such an extended foil target sufficiently close to the hot spot to limit time-of-flight dispersion of the ignitor power will require cone-guiding through the fuel capsule [40], with a wide cone aperture. A conically guided capsule will also limit the implosion driver energy while largely preserving the gain [40].

With a 300 kJ ignitor and the highest reported laser-to-proton energy conversion efficiency, 15% [41, 42], an overall laser energy of 2 MJ will be needed to drive the ignitor. This energy will have to be delivered to the foil target over a timescale of 1 ps. Suitable laser amplifiers and laser architectures will have to be developed to this extent as well as for the ns-scale implosion of the fuel, where driver energies above 10 MJ are expected. Both Diode-Pumped Solid-State Laser (DPSSL) and excimer laser systems show the potential to be scaled up to the large energy outputs required for compression and fast ignition of H11B fuel, on both the ns and ps timescales [43, 44].

We finally recall that within the frame of a very specific fast ignition scheme, based on a laser-driven relativistic shock wave, Eliezer et al. [45] have found that a laser pulse with intensity of 1.6 × 1025 W/cm2, duration of 1 ps and energy of 21 MJ impinging on fuel pre-compressed at 4,800 g/cm3 can generate a side, cylindrical hot spot with a depth of 8.3 g/cm2, Ti200 keV, Te50 keV, where ignition is achieved. Such a laser pulse is judged impracticable in the near term.

On the contrary, our preliminary analysis shows that proton fast ignition of isochoric H11B fuel requires compression and ignitor performances which, though challenging, are in line with near-future laser capabilities. We plan to devote further work to demonstrate burn propagation, better quantify ignition parameters and calculate gain in such scheme, considering actual target configurations.

Data availability statement

The original contributions presented in the study are included in the article/Supplementary Material, further inquiries can be directed to the corresponding author.

Author contributions

EG: Formal Analysis, Writing–original draft, Writing–review and editing, Data curation, Investigation, Software, Visualization. FB: Formal Analysis, Writing–original draft, Writing–review and editing, Conceptualization, Methodology, Supervision, Validation.

Funding

The author(s) declare that financial support was received for the research, authorship, and/or publication of this article. HB11 Energy Ltd. Pty. has supported this work through the consultancy contract of the first author and the payment of the publishing fee. This work has been carried out under the Collaborative Science Program of HB11 Energy.

Acknowledgments

The authors wish to thank D Batani, S Pikuz, E Turcu and D Margarone for useful discussions. The authors are indebted with I Morozov for an independent verification of their results. FB is grateful to F Ladouceur for hosting his fellowship at UNSW Sydney.

Conflict of interest

Author EG was affiliated to HB11 Energy Holdings Ltd Pty.

The remaining author declares that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.

The authors declare that this study received funding from HB11 Energy Pty. Ltd. The funder was involved in the discussion of the results and in the decision to submit the manuscript for publication.

Publisher’s note

All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations, or those of the publisher, the editors and the reviewers. Any product that may be evaluated in this article, or claim that may be made by its manufacturer, is not guaranteed or endorsed by the publisher.

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Appendix A: Formalism

Power density terms

Explicit expressions for the power density terms in Eqs 16 are given hereafter (electrostatic cgs units are used):

Pth=npnBσvQ(A1)

where σv is the Maxwellian reactivity [28];

Pb=8.511W0Te^1/2{Zeff1+1.78Te^1.34+2.12Te^1+1.1Te^+Te^21.25Te^2.5}(A2)

where Te^=kTe/mec2 and W0=e6ne2/mec2ħ [6, 46];

Pie=32npνpe+nBνBekTiTe(A3)

where νie=νie*,

νie*=4π2nee4Zi2lnΛie32π3/2mimemekTe3/2(A4)

is the classical heat exchange rate [29],

=1+2Te^+2Te^2πTe^3/20exp{1+x21/Te^}x2dx(A5)

is its relativistic correction [6], and

lnΛie=32Zie34.2×105kπnekTe(A6)

according to Spitzer [47];

Ph=ϵZiκTeS/V(A7)

where TeTe/R, S is the area of the hot-spot surface (S/V=3/R),

κ=202π3/2kT5/2kme1/2e4ZilnΛieδTZi(A8)

is the Spitzer thermal conductivity, with ZiZeff for a multi-Z plasma, and the correction factors ϵ and δT have been calculated through interpolation (ϵ=0.407, δT=0.426) [47];

Pm=Pm,i+Pm,e(A9)
Pm,ie=3pieRu(A10)

where u3p/4ρ is the velocity of the material behind a strong shock in isochoric fuel [35] and the pressures p, pi, pe are given by Eqs 1012.

Fusion energy partition and stopping power

The fusion power fraction to ions, ηi, has been calculated according to Levush and Cuperman [48] (Figure A1). A stopping power of the form

dE/dt=E/tE+γ/E(A11)

has been used for the fusion-born α particles, with tE and γ given by Corman et al. [49]. A simplified α spectrum has been utilised, as explained in Ref. [20]. ηi approaches or even overcomes 90% at values of Ti and Te of interest for ignition and burn. The same stopping power model of Eq. A11 has been utilised for energy-range calculations for the ignitor protons.

FIGURE A1
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FIGURE A1. Fusion power fraction to ions (electrons) as a function of Ti, with Te=Ti/2. Calculations are made for ni=1026/cm3, ε=0.15, and depend on density weakly.

Useful relations

The densities np and nB are linked to ne and ρ by the obvious relations

np=ne/Zp+εZB(A12)
nB=εne/Zp+εZB(A13)
ne=Zni(A14)
ρ=niAmp(A15)

with Z and A given by Eq. 8.

Keywords: proton-boron fusion, inertial confinement fusion, hot-spot ignition, proton fast ignition, laser boron fusion, aneutronic fusion

Citation: Ghorbanpour E and Belloni F (2024) On the ignition of H11B fusion fuel. Front. Phys. 12:1405435. doi: 10.3389/fphy.2024.1405435

Received: 22 March 2024; Accepted: 24 June 2024;
Published: 05 August 2024.

Edited by:

Eliezer Shalom, Soreq Nuclear Research Center, Israel

Reviewed by:

Zohar Henis, Soreq Nuclear Research Center, Israel
Dimitri Batani, Université de Bordeaux, France
Fuyuan Wu, Shanghai Jiao Tong University, China

Copyright © 2024 Ghorbanpour and Belloni. This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.

*Correspondence: Fabio Belloni, Zi5iZWxsb25pQHVuc3cuZWR1LmF1

Present address: Fabio Belloni, European Commission, Directorate-General for Research and Innovation, Euratom Research, Brussels, Belgium

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