AUTHOR=Subramanian Arunprabaharan , Azimi Mona , Leong Cheng Yee , Lee Siew Ling , Santato Clara , Cicoira Fabio TITLE=Solution-Processed Titanium Dioxide Ion-Gated Transistors and Their Application for pH Sensing JOURNAL=Frontiers in Electronics VOLUME=3 YEAR=2022 URL=https://www.frontiersin.org/journals/electronics/articles/10.3389/felec.2022.813535 DOI=10.3389/felec.2022.813535 ISSN=2673-5857 ABSTRACT=

Titanium dioxide (TiO2) is an abundant metal oxide, widely used in food industry, cosmetics, medicine, water treatment and electronic devices. TiO2 is of interest for next-generation indium-free thin-film transistors and ion-gated transistors due to its tunable optoelectronic properties, ambient stability, and solution processability. In this work, we fabricated TiO2 films using a wet chemical approach and demonstrated their transistor behavior with room temperature ionic liquids and aqueous electrolytes. In addition, we demonstrated the pH sensing behavior of the TiO2 IGTs with a sensitivity of ∼48 mV/pH. Furthermore, we demonstrated a low temperature (120°C), solution processed TiO2-based IGTs on flexible polyethylene terephthalate (PET) substrates, which were stable under moderate tensile bending.