- 1Key Laboratory of Petroleum Resources Research, Institute of Geology and Geophysics, Chinese Academy of Sciences, Beijing, China
- 2College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing, China
- 3Innovation Academy for Earth Science, Chinese Academy of Sciences, Beijing, China
The Shenhu area of the South China Sea (SCS) is one of the most promising fields for natural gas hydrate (NGH) exploitation. However, previous studies conclude that using only depressurization is inefficient for this challenging hydrate deposits surrounded by permeable water zones, which requires assistance by thermal stimulation to promote hydrate decomposition and methane recovery. However, traditional thermal stimulation methods with hot water or steam injection induce massive heat loss along the wellbore. In addition, in situ electrical heating only results in a limited high temperature region due to low thermal conductivity of hydrate deposits. Therefore, we numerically investigate the performance of combined brine flooding with electrical heating–assisted depressurization in horizontal wells for exploitation of natural gas hydrate in the SCS, which simultaneously possesses the merits of low heat loss and enhanced heat transfer by convection. Our simulation results show that thermal stimulation by combined brine flooding with electrical heating can significantly enhance hydrate dissociation and methane recovery. After 20 years of production, the cumulative methane production of combined brine flooding with electrical heating–assisted depressurization is 1.41 times of that conducted by the only depressurization method. Moreover, the energy efficiency can be improved by reducing electrical heating time, and terminating electrical heating with 70% hydrate dissociation achieves the highest net energy gain. In addition, methane recovery and net energy gain increases with electrical heating power and brine injection pressure but with a decreasing rate. Therefore, the selection of electrical heating power and brine injection pressure should be performed carefully and comprehensively considering both the efficiency of gas production and risks of geological hazard. It is hoped that our research results will provide reference and guidance for the development of a similar NGH reservoir in order to promote the industrial development process of NGH.
Introduction
Natural gas hydrates are crystalline substances comprising water molecules and gas molecules, in which a solid water lattice accommodates gas molecules in a cage-like structure (Sloan, 2003; Wang et al., 2017; Wu et al., 2020). The most typical hydrate-forming gas is methane, and NGH mainly occurs in terrestrial permafrost and offshore sediments where low temperature and high-pressure conditions needed by hydrate stabilization are met (Collett, 2002; Koh, 2002; Chong et al., 2016). As a potential new unconventional energy, NGHs are currently attracting significant attention owing to their extensive distribution, great resource potential, high energy density, and low environmental pollution (Koh et al., 2012; Yang et al., 2018). Current estimations of the hydrate-containing hydrocarbon gas available at standard conditions ranges from 1015 to 1018 m3, which is twice as much as the conventional fossil energy (Moridis et al., 2009a). If NGH can be exploited in a safe and efficient way to produce natural gas and replace traditional fossil fuels, the problem of global energy shortage and environmental pollution can be greatly alleviated (Liang et al., 2020; Yin et al., 2020).
The Shenhu area on the northern continental slope of the South China Sea (SCS) is one of the most promising fields for gas hydrate exploitation. In 2007, 2015, and 2016, three gas hydrate drilling expeditions (GMGS1, 3, and 4) were conducted in this area by the Guangzhou Marine Geological Survey (Wu and Wang, 2018). During the GMGS1, five sites were selected for deep drilling and sampling in the Shenhu area (Figure 1), among which three sites (SH2, SH3, and SH7) were verified with the existence of methane gas hydrates by depressurization experiments (Wu et al., 2011). Since then, many numerical simulations were carried out on hydrate production in the Shenhu area, including the SH2 site (Su et al., 2011; Su et al., 2012b; Su et al., 2013; Jin et al., 2016), SH3 site (Su et al., 2012a), and SH7 site (Li et al., 2010; Li et al., 2011; Li et al., 2013; Sun et al., 2015). These simulations include different production methods, such as depressurization and thermal stimulation, the use of vertical and horizontal wells, the effects of the underlying and overburden layer permeability, and other aspects related to hydrate production (Sun et al., 2019). Based on aforementioned numerical studies and many other laboratory experiments on the NGH in the SCS, the China Geological Survey successfully conducted the first and second production tests in the Shenhu area of the SCS in 2017 and 2020, respectively, using a vertical well and a horizontal well. The first production test lasted for 60 days with a cumulative gas production of 3.09 × 105 m3 (Li et al., 2018b), and the second production test achieved 30 days of continuous gas production, with a cumulative gas production of 8.614 × 105 m3, whose average daily gas production is 5.57 times as much as that obtained in the first production test (Ye et al., 2020). The two successful production tests proved the technical feasibility of gas production from the clayey silt NGH reservoir, which accounts for 90% of the total hydrate reservoirs but tend to be the most difficult to exploit owing to low permeability and high content of clay (Boswell and Collett, 2011).
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FIGURE 1. Location of study area, drilling sites, and the confirmed gas hydrate distribution in the Shenhu area. Insert: General location of study area in the northern slope of the South China Sea (Wu et al., 2011).
To exploit the NGH, the equilibrium state of the reservoirs should be broken by certain mechanisms, leading to in situ dissociation of the NGH into gas and water; then the gas–water mixture can be extracted and gas–liquid separation can be conducted successively (Konno et al., 2016). According to the phase equilibrium curve of the NGH, those certain mechanisms include the following: depressurization (Moridis et al., 2007; Moridis et al., 2009b; Sun et al., 2015; Yang et al., 2019); thermal stimulation (Moridis et al., 2004; Wang et al., 2018; Liu et al., 2020); use of inhibitors (Sung et al., 2002); and gas molecule exchange (White et al., 2011; Koh et al., 2016; Zhang et al., 2017). Currently, depressurization is considered to be the most economical and efficient method for NGH exploitation (Oyama et al., 2012; Chong et al., 2017), which was used in the first and second production tests in the Shenhu area of the SCS. However, there are also problems attached to this method, such as small influence range and rapid drop of the gas production rate. Hydrate decomposition is an endothermic reaction, but the only heat sources of NGH exploitation by depressurization are the sensible heat of the hydrate deposit, the heat transferred from the surroundings, and the latent heat released by the phase transition from water to ice (Zhao et al., 2014). Due to insufficient heat supply, the reservoir temperature will significantly reduce which may lead to the formation of ice and secondary hydrate, hindering the recovery of methane (Wang et al., 2020). Therefore, thermal stimulation methods are usually used in company with depressurization to provide additional heat for the hydrate deposit and accelerate NGH dissociation (Wan et al., 2018).
Traditional thermal stimulation methods utilize hot water and steam injection, which can be implemented in the form of the huff and puff method, hot water/steam flooding, and hot water/steam-assisted gravity drainage (SAGD). Actually, these methods have widely been used in the field of thermal enhanced oil recovery and provide a significant amount of oil in the overall global oil outlook (Mokheimer et al., 2019). Many authors also evaluated the potential of these methods in promoting methane production from the NGH by laboratory experiments and numerical simulations. Li et al. (2011) and Su et al. (2012b) numerically investigated the gas production performance by the huff and puff method in the Shenhu area, and the results showed that the gas production rate was very low and the secondary hydrate formation occurs during the injection stage. In addition, Feng et al. (2013) and Feng et al. (2014) compared the gas production potential of depressurization combined with warm brine injection by different dual horizontal well configurations, respectively, corresponding to the flooding method (dual horizontal wells in the same horizontal plane) and the SAGD method (dual horizontal wells in the same vertical plane). They concluded that the average gas production rate of the flooding method exceeds the commercially viable production rate in the Gulf of Mexico, which is more favorable than the SAGD method. In addition, Jin et al. (2016) also proved that gas recovery can be improved significantly by hot water flooding for the hydrate deposits in the Shenhu area, and the well spacing affects the methane production significantly when thermal stimulation starts. However, when hot water or steam is injected, the heat loss along the wellbore is considerable even with insulated tubing, after hundreds or even thousands of meter transportation from the surface or ocean to the hydrate-bearing layers (hereafter, referred to as HBL) (Li et al., 2018a).
To overcome the shortcoming of traditional hot water/steam flooding method, novel thermal stimulation methods of electrical or electromagnetic heating and methane in situ combustion have been proposed, which generate heat directly in the formation to avoid wellbore heat loss. In this study, we focus on electrical heating, and many laboratory experiments have been conducted to clarify the effects of electrical heating–assisted depressurization on hydrate dissociation and methane recovery (Falser et al., 2012; Li et al., 2018a; Liang et al., 2018; Minagawa et al., 2018; Wan et al., 2020a; Wan et al., 2020b; He et al., 2021). For example, Li et al. (2018b) found that the production efficiency of depressurization can be greatly enhanced by using the electrical heating simultaneously for the methane hydrate in a cuboid pressure vessel. In their experiment, a resistance heating wire is distributed uniformly in the inner surface of the well, and the whole well can be heated evenly when direct current is supplied to the wire. On the other hand, electrical heating was performed through the application of alternating current using two end caps as a pair of electrodes in the experiments by Minagawa et al. (2018), which suppressed the decrease in the temperature of NGH sediment core and enabled higher gas production when combined with depressurization. In addition, Wan et al. (2020b) proposed a novel tripartite strategy of electrical resistance heating, room temperature water flooding, and depressurization which combines the advantages of simultaneously reducing heat loss and enhanced heat transfer by convection and results in the best energy recovery efficiency among different thermal stimulation modes in a high-pressure reactor using two vertical wells. In addition to laboratory experiments, several numerical simulations were also conducted on the gas production of hydrate dissociation by electrical heating combined with depressurization (Wan et al., 2020a; Li et al., 2020; Zhao et al., 2021; Liu et al., 2022), but mainly performed in the laboratory scale. Wan et al. (2020a) conducted simulations of wellbore heating with depressurization for gas production from hydrate sediments in a rectangular cylinder model. Their results showed that a combination of depressurization and wellbore heating is more favorable for the enhancement of heat transfer and faster energy recovery. Similarly, in a laboratory-scale axisymmetric model, Liu et al. (2022) conducted simulations on the gas production behavior from the depressurization-induced dissociation of methane hydrate by electrical heating and on the optimization of the electrical heating scheme to achieve high-efficient utilization of electrical energy. However, the numerical simulations in the reservoir scale are rare, and recently Zhao et al. (2021) numerically evaluated the production performance of the low-frequency electrical heating–assisted depressurization (LF-EHAD) method for methane recovery from hydrate deposits in the Shenhu area of the SCS. In addition, the LF-EHAD method significantly enhances hydrate dissociation and gas production over the depressurization method and outperforms hot water flooding in higher energy utilization efficiency. Due to the large gap between laboratory and reservoir conditions, it is necessary to further numerically investigate the methane production from the NGH by electrical heating–assisted depressurization in field scale.
Therefore, the goal of this study is to numerically evaluate the performance of the combined brine flooding with electrical heating–assisted depressurization for hydrate exploitation in the Shenhu area of the SCS. The tripartite exploitation strategy with brine injection given by Wan et al. (2020b) is utilized because the simulation results of hydrate exploitation in field scale by in situ electrical heating show limitation of the high- temperature region and existing mainly near the heating wellbore due to the low thermal conductivity of hydrate deposits (Li et al., 2020). In consideration of the obvious advantages of horizontal wells over vertical wells, such as increasing single-well controlled reserves and gas production and reducing the risks of generating secondary hydrates and freezing (Feng et al., 2015; Ye et al., 2020), we adopt the same well configuration as done by Feng et al. (2014), that is, horizontal wells in the same horizontal plane. In addition, the pure depressurization method is also conducted as a comparison. In order to optimize the novel tripartite strategy, numerical results of methane recovery, water production and energy efficiency from different electrical heating times and power, and brine injection pressure are provided in detail and comprehensively analyzed. It is hoped that our numerical results in this study will provide reference and guidance for the development of similar low-permeability marine clayey–silt NGH with permeable surrounding water zones.
Materials and Methods
Geological Setting of Study Area
The Shenhu area is near southeast of Shenhu Underwater Sandy Bench in the middle of the north slope of the SCS, between Xisha Trough and Dongsha Islands. Tectonically, the research area is located in the Zhu II Depression, Pearl River Mouth Basin (Figure 1), which has been in the process of tectonic subsidence since the middle Miocene along with a high sedimentation rate, providing abundant organic matter (producing methane by pyrolysis or biological action) for the NGH (Wu et al., 2010). Large-scale mud diapirs, vertical fissure systems, and highly angled fractures were formed by tectonic movements, which can provide conduits for gas migration (Sun et al., 2019). The bottom temperature of the Shenhu area is 3.3–3.7°C with a geothermal gradient of 45–67°C/km, and the bottom pressure is more than 10 MPa (Yang et al., 2010; Sun et al., 2015), which meets the favorable temperature and pressure conditions for the formation of the hydrate reservoir. Therefore, this area becomes one of the most promising fields for gas hydrate exploitation.
In this study, we focused on the hydrate deposits that occur at the site SH2 drilled in GMGS1 because of high hydrate saturation and substantial amount of available data. The water depth at SH2 is 1,235 m. The HBL is 40 m thick overlain by a permeable overburden of 188 m thick and underlain by a permeable zone of mobile water. Based on the drilling and sampling data, the hydrate saturation ranges from 25 to 48%, and the porosity ranges from 0.33 to 0.48, which implies that a huge amount of natural gas is stored in the hydrate deposits. The hydrate disseminates in the sediments that mainly comprise silty clay and clay silt. In addition, it is detected that the gases contained in the hydrate in SH2 mainly consist of methane (96.10–99.91%) with minor quantities of ethane and propane (Wu et al., 2010).
Model Setup and Well Configuration
Based on the geological setting of SH2 of the Shenhu area in the SCS, the established conceptual model for numerical simulation and well configuration is shown in Figure 2A. The conceptual model consists of three horizontal layers including the 40-m-thick HBL and 30-m-thick permeable overburden and underburden water-bearing stratums (100 m in total), which are thought to be sufficient to accurately calculate the heat transfer to the HBL during the 20 years of production (Moridis and Reagan, 2011). The hydrate in the HBL is assumed to only comprise methane with a saturation of 0.4, and the remaining pore space is occupied by water with a saturation of 0.6. The porosity and intrinsic permeability of the HBL are, respectively, 0.38 and 10 millidarcy (mD). Due to lack of relevant information, the lithology of the surrounding water-bearing stratums is assumed to be same as the HBL but lacking hydrate. The values of simulation parameters used in our numerical model are summarized in Table 1.
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FIGURE 2. Schematic diagrams of (A) the conceptual model and the well configuration and (B) domain discretization mesh used in our numerical simulations. The outside of the middle well is surrounded by the electric resistance wire which can release heat when current flows by.
As shown in Figure 2A, three horizontal wells are adopted in our study considering their obvious advantages over vertical wells, such as increasing single-well controlled reserves and gas production and reducing the risks of generating secondary hydrates and freezing (Feng et al., 2015; Ye et al., 2020). In order to avoid water and gas leakage, the vertical part of wells is sealed and the opened horizontal part with a length of 1,000 m is located at the middle of the HBL. Same as the study by Moridis et al. (2013), the interior of the wells is defined as pseudo porous media approximately, which has a high porosity of 1.0, a high permeability of 1.0 × 10−6 m2, and a low capillary pressure of 0. Two side wells are conducted at a constant pressure to produce methane for the whole exploitation period (20 years). However, the middle well is first used to depressurize for 5 years in order to dissociate the hydrate and increase the permeability around the well. Then, thermal simulation starts by the flowing electric current through the resistance wire around the middle well. At the same time, a brine of 20°C (directly from sea) is also injected into hydrate formation at a constant pressure by the middle well, which can carry the electrical heat deep into the HBL.
A unit width (1 m) in y direction is used without considering the pressure and temperature drop in the wellbore of the horizontal wells. In addition, a mild well spacing of 75 m is adopted, considering that small well spacing controls less reserves and big well spacing may go beyond the influence radius of the injected electrical heat (Jin et al., 2016). In addition, due to symmetric well configuration, only half of the hydrate deposits need to be simulated. Therefore, the size of the 2D numerical model is 75 m × 100 m in x and z directions, which is discretized into 101 × 114 = 11,514 grid blocks (Figure 2B). Because the vicinity of the wellbore had been shown to be critically important to production (Moridis et al., 2009b), a very fine discretization of 0.25 m was used around the horizontal wells. In addition, the spacing intervals increase with the distance to wells, which reaches a size of 2 m at the middle between the wells and at the top and bottom of the model.
The numerical simulator used for the simulation of the behavior of hydrate-bearing geologic systems in this study is TOUGH + HYDRATE, which was developed by the Lawrence Berkeley National Laboratory (Moridis, 2014). The initial distributions of pressure and temperature are, respectively, obtained by hydrostatic pressure distribution and a geothermal gradient of 0.047°C/m (Moridis et al., 2007; Su et al., 2012b). In addition, the base of the HBL initially lies in the hydrate equilibrium condition. As for boundary conditions, constant temperature and pressure boundary are applied to the top and the bottom of the model, and non-flow boundary is applied at x = 0 and x = 75 m during the whole exploitation period (Su et al., 2012a, 2012b; Li et al., 2013).
Simulation Scenarios
The factors that are related to gas production performance of a hydrate deposit can be divided into two classes: formation conditions and artificial operations. The most related formation condition is the permeability of the HBL, which can be improved by hydraulic fracturing, but not involved in our research. Therefore, we mainly consider optimizing artificial operations to promote the exploitation of the NGH, including electrical heating time and power and brine injection pressure, whose effects to gas production are investigated by different exploitation scenarios listed in Table 2. As the base case, A0 adopts a brine injection pressure of 17 MPa, which corresponds to the maximum of the wellbore pressure to avoid the overpressure of the HBL (Li et al., 2011). In addition, 2,000 W of electrical heating is applied to the same 2D-simulated hydrate deposit of 75 m × 100 m. In addition, the only depressurization method D1 is also included to verify the feasibility of the new exploitation method of combined brine flooding with electrical heating–assisted depressurization. The production pressures of all scenarios are set to be 8 MPa, which is larger than the pressure at the quadruple point to eliminate the possibility of ice formation.
The following criteria are used to compare the gas production performance of different exploitation scenarios: volumetric rate of total produced methane from wells (QP) and volumetric rate of produced methane in gas phase (QPG), volumetric rate of released methane by hydrate dissociation (QR), and volumetric rate of produced water (QW); cumulative volume of methane and water produced from wells (VP and VW, respectively), gas-to-water ratio (RGW); energy efficiency ratio (η) and net energy gain (Enet). Among these criteria, four of them are particularly important, which can also be classified as relative criterion (RGW and η) and absolute criterion (VP and Enet), which are also listed in Table 2. RGW is defined as the ratio of VP and VW, while η is the ratio of the recovered energy to the total consumed energy, which can be defined as
where
In order to simulate actual exploitation conditions, all of these criteria are scaled according to the length of the horizontal wells (1,000 m).
Results and Discussion
Effects of Combined Brine Flooding With Electrical Heating
The exploitation scenario of pure depressurization is first simulated and evaluated, whose methane volumetric rate and water production are shown in Figure 3. As shown in Figure 3A, the hydrate is rapidly dissociated by depressurization in the initial stage due to the largest pressure difference between production wells and formation, known as pressure driving force. Therefore, QR and QP, respectively, reach a maximum of 260,000 m3/day and 43,000 m3/day in a short time. In addition, QR is larger than QP in the first 580 days, indicating that the released methane cannot be produced in time due to the low permeability of the HBL. With the reduction of pressure driving force and exhaustion of the hydrate around production wells, QR rapidly drops below QP, and the remaining methane is discharged from production wells. Then, QP and QR almost keep stable before a sudden decrease happening at 5 years. The reason is that the hydrate between the HBL and surrounding permeable water-bearing stratums is completely dissociated, resulting in rapid water invasion, proven by the sudden increase of the water-produced rate (QW) at 5 years in Figure 3B. Massive water production slows down the propagation of low pressure. Therefore, QP and QR keep decreasing with a similar trend and reach a value of 6,500 m3/day at the end of simulation, which is much lower than the commercially viable production rate.
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FIGURE 3. Evolution of (A) methane production rate (QP), methane production rate in gaseous phase (QPG) and release rate (QR), (B) water production rate (QW) and water production volume (VW) for the only depressurization method and combined brine flooding with electrical heating–assisted depressurization method (the base-case). The unit of the volumetric rate is measured at standard temperature and pressure.
However, QW keeps increasing in the whole simulation process due to increase of formation permeability after hydrate dissociation and the influence of permeable water-bearing stratums. The different variations of QP and QW indicate that gas production is controlled by methane from hydrate dissociation rather than original methane dissolved in in situ water. In addition, the released methane can be produced in free gas or in dissolution. Initially, due to rapid release of methane from hydrate dissociation, free gas takes a large proportion of the total produced methane. However, QG gradually decreases with reduction of QR and becomes zero at 2,650 days, indicating that methane is produced completely in dissolution after then. The relative criterion (RGW and η) and absolute criterion (VP and Enet) to judge gas production performance are given in Figure 4. At the end of the simulation, the cumulative volume of the produced methane for only depressurization is 9.7 × 107 m3, corresponding to an average production rate of 13,275 m3/day. With the increase of the produced water rate and the decrease of produced methane rate, RGW and η of only depressurization keeps descending, respectively, with a final value of 2.20 and 5.65.
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FIGURE 4. Evolution of (A) methane production volume (VP) and gas-to-water ratio (RGW), (B) energy efficiency ratio (η) and net energy gain (Enet) for the only depressurization method and combined brine flooding with electrical heating–assisted depressurization method (the base-case).
From the previous analysis, only depressurization is inefficient for the challenging hydrate deposit with permeable overlying and underlying layers. The hydrate dissociation rate and methane production rate will rapidly decrease when the water from the surrounding permeable layers invades into the HBL. Therefore, thermal stimulation by combined brine flooding with electrical heating is conducted after 5 years of only depressurization in order to promote hydrate dissociation. For the base case, brine injection (20°C) at a constant pressure of 17 MPa and electrical heating with a power of 2,000 W are simultaneously applied to the left well, while the other well is still used for depressurization at a constant pressure of 8 MPa. For comparison with only depressurization, methane production, water production, and energy gain of the base case are also given in Figures 3, 4. In addition, Figures 5–8, respectively, show the evolution of temperature (T), hydrate saturation (SH), gas saturation (SG) and salinity (Xinh) of the base case in order to figure out the variation of the system state over time under thermal stimulation.
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FIGURE 5. Evolution of spatial distributions of temperature (T) over time: (A) 5 years, (B) 7 years, (C) 9 years, (D) 12 years, (E) 16 years, and (F) 20 years for the combined brine flooding with electrical heating–assisted depressurization method (the base-case).
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FIGURE 6. Evolution of spatial distributions of hydrate saturation (SH) over time: (A) 5 years, (B) 7 years, (C) 9 years, (D) 12 years, (E) 16 years, and (F) 20 years for the combined brine flooding with electrical heating–assisted depressurization method (the base-case).
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FIGURE 7. Evolution of spatial distributions of gas saturation (SG) over time: (A) 5 years, (B) 7 years, (C) 9 years, (D) 12 years, (E) 16 years, and (F) 20 years for the combined brine flooding with electrical heating–assisted depressurization method (the base-case).
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FIGURE 8. Evolution of spatial distributions of salinity (Xinh) over time: (A) 5 years, (B) 7 years, (C) 9 years, (D) 12 years, (E) 16 years, and (F) 20 years for the combined brine flooding with electrical heating–assisted depressurization method (the base-case).
When thermal stimulation starts at 5 years, QR of the base case rapidly increases and reaches a peak of 45,000 m3/day, proving that hydrate dissociation is accelerated by the electrical heat, which is carried by the brine into the deep of the HBL. On the other hand, the vacated pore space after hydrate dissociation increases the permeability of formation, which is beneficial to the flow of the heated brine. As a result, hydrate complete dissociation area and high-temperature region around the injection well move rapidly toward the production well (Figures 5, 6). Contrary to the immediate increase of QR, QP and QPG first drop by half after thermal stimulation due to the halving of production wells and then keep decreasing until 3,280 days. During this stage, the released methane is detained in the HBL due to the distance between the wells, which leads to the increase of gas saturation (Figures 7A,B). Therefore, further dissociation of the hydrate is suppressed, and QR gradually decreases.
When the released methane reaches the production well at 3,280 days (Figure 7C), QP and QG start rapidly increasing, which is 1,455 days later than the increase of QR. Then, QP exceeds QR at 4,420 days and reaches a peak of 6,140 m3/day at around 6,000 days, indicating that the detained methane is gradually produced. After 6,000 days, a quick drop of QR (as well as QP and QPG) appears due to the exhaustion of the hydrate, validated by the small green part in Figures 6E,F. In addition, the similar variation between QP and QPG indicates that gaseous methane makes the main contribution of the increase of QP after thermal stimulation. As shown in Figure 8, a high salinity abnormal forms at the behind of the dissociation interfaces around the injection well. This is a sign of secondary hydrate formation because that salt is excluded from the lattice of the hydrate, which originates from the pressure increment by brine injection and should be responsible for the fluctuations of QR after thermal stimulation. With the exhaustion of the hydrate, the high salinity abnormal gradually disappears.
Different from the continuous increase of the water production rate of only depressurization, water production of the base case is suppressed when the released methane reaches the production well, because the relative permeability of water is inversely proportional to gas saturation. With the discharge of methane and increase of absolute permeability of formation, QW increases again after 5,500 days but is still much lower than that of only depressurization. From Figure 4A, thermal stimulation by combined brine flooding with electrical heating can greatly increase methane recovery, with a higher VP (except the period before methane reaches production well) and RGW over only depressurization. At the end of the simulation, the cumulative volume of the produced methane is increased by 41% with thermal stimulation. However, the net energy gain of the base case shows no improvement over only depressurization because the additional methane recovery is offset by massive injected electrical heat, and a rather low energy efficiency ratio of 2.33 is obtained by thermal stimulation. Therefore, the energy efficiency of the combined brine flooding with electrical heating–assisted depressurization needs to be improved before field application.
Sensitivity Analysis of Electrical Heating Time
In order to save energy and gain a higher energy efficiency, electrical heating should be terminated at the later stage of the base case because there is only little hydrate left (Figures 6E,F). Therefore, another two runs of A1 and A2 are conducted to determine the effects of the electrical heating time, which, respectively, terminate electrical heating when the rate of the dissociated hydrate to the initial hydrate (SR) reaches 0.5 (at 3,156 days) and 0.7 (at 4,579 days). The base case corresponds to an SR of 1.0, which means that electrical heating lasts until the end of the simulation. Though electrical heating stops at an earlier time for A1 and A2, brine of 20°C is still injected into the HBL with an injection pressure of 17 MPa to assist the drainage of methane. As shown in Figure 9A, longer electrical heating time leads to a higher QP due to more hydrate dissociation. In addition, the termination of electrical heating results in the increase of QW on account of the alleviation of water production restriction by the reduction of gas saturation around the production well (Figure 9B). However, QW increases with increasing of SR at the end of the simulation because more vacated pore space for a longer electrical heating time leads to higher formation permeability. In addition, the final VW is almost equal for different electrical heating times.
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FIGURE 9. Evolution of (A) methane production rate (QP), (B) water production rate (QW) and water production volume (VW), (C) methane production volume (VP) and gas-to-water ratio (RGW), and (D) energy efficiency ratio (η) and net energy gain (Enet) under different electrical heating times.
The optimization of electrical heating time can be achieved by the criteria shown in Figures 9C,D. Compared with the base case, VP only decreases by 5.1%, but the injected heat is reduced by 49.7% for terminating electrical heating when 70% hydrate has already been dissociated (SR = 0.7). Therefore, the energy efficiency and net energy gain can be greatly improved by decreasing electrical heating time. However, further advancing the termination of electrical heating with an SR of 0.5 decreases VP by 16.1%, and the net energy gain is lower than that of terminating electrical heating with an SR of 0.7, indicating that stopping electrical heating prematurely is disadvantageous to methane production due to insufficient hydrate dissociation, even though a higher energy efficiency ratio is obtained. Therefore, a medium electrical heating time is preferred for gas production from hydrate deposit in order to accelerate hydrate dissociation and gain satisfactory energy efficiency. Thus, the subsequent simulations all terminate electrical heating when 70% of hydrate is dissociated in order to avoid massive energy waste.
Sensitivity Analysis of Electrical Heating Power
Apparently, the gas production performance of the combined brine flooding with electrical heating–assisted depressurization is closely related to electrical heating power. Therefore, another two simulations with a power of 1,000 W (B1) and 3,000 W (B2) are conducted to explore the effects of electrical heating power. The two additional simulations adopt same parameters as A2 except the electrical heating power, which also terminate electrical heating when 70% hydrate has already been dissociated in order to save energy. As shown in Figure 10A, QP initially increases with electrical heating power because of the accelerated hydrate dissociation. Moreover, a larger power not only induces earlier increase of QP due to advanced breakthrough of released methane from the injection well to the production well but also induces earlier drop of QP due to the advanced termination of electrical heating. In addition, faster exhaustion of the hydrate induces that QP decreases with increasing of the electrical heating power at the end of the simulation. Contrary to QP, a larger power leads to a lower QW at an early time and a higher QW at a later time (Figure 10B). The different variation of methane production and water production is reasonable considering that the relative permeability of gas phase and aqueous phase change oppositely at all times. In addition, the final VW is basically unchanged with electrical heating power.
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FIGURE 10. Evolution of (A) methane production rate (QP), (B) water production rate (QW) and water production volume (VW) under different electrical heating powers, (C) methane production volume (VP) and gas-to-water ratio (RGW), and (D) energy efficiency ratio (η) and net energy gain (Enet) under different electrical heating powers.
The relative criteria and absolute criteria are also given in Figures 10C,D in order to optimize the electrical heating power. From Figure 10C, VP and RGW increase with the electrical heating power though with a decreasing rate. Compared with the electrical heating power of 2,000 W, VP increases by 5.9% for the electrical heating power of 3,000 W, while VP decreases by 12.0% for the electrical heating power of 1,000 W. Thus, a low electrical heating power of 1,000 W is inefficient for gas production from the hydrate deposit though with a high energy efficiency ratio (Figure 10D). In addition, the net energy gain of 2,000 and 3,000 W is basically the same, indicating that the additional recovered methane just catches up with the enlarged electrical heat injection. At the same time, increasing electrical heating power also enlarges the risks of wellbore failure due to thermal stress variation. Therefore, a mild electrical heating power is preferred for increasing methane recovery and reducing geological risks.
Sensitivity Analysis of Brine Injection Pressure
Other than electrical heating power, brine injection pressure is also a key parameter related to gas production performance, whose effects are determined by another two procedures with injection pressure of 15 MPa (C1) and 19 MPa (C2). Except brine injection pressure, other parameters of C1 and C2 are the same as A2. From the simulation results of methane and water production shown in Figures 11A,B, QP initially increases with injection pressure because of faster brine injection, leading to a larger heat diffusion rate. Driven by larger pressure gradient between wells, faster breakthrough of released methane is also realized by higher injection pressure. At the same time, the advanced termination of electrical heating after 70% of hydrate dissociation for higher injection pressure induces an earlier drop and a lower final value of QP. As clarified before, QW still varies oppositely with QP. However, a confusing phenomenon of water production is that larger injection pressure, instead, possesses a lower final VW. This can be explained as more methane accumulation around the production well by higher injection pressure results in a stronger suppression of water production in the early stage of the thermal stimulation.
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FIGURE 11. Evolution of (A) methane production rate (QP), (B) water production rate (QW) and water production volume (VW), (C) methane production volume (VP) and gas-to-water ratio (RGW), and (D) energy efficiency ratio (η) and net energy gain (Enet) under different brine injection pressures.
The superiority of higher brine injection pressure is adequately verified by higher methane recovery and gas-to-water ratio (Figure 11C), as well as the higher energy efficiency ratio and net energy gain (Figure 11D). Raising brine injection pressure from 15 to 17 MPa increases Enet by 60.4%, while further raising injection pressure to 19 MPa only increases Enet by 8.0%. On the other hand, higher injection pressure also enlarges the risks of geological hazards, such as reservoir instability and submarine landslide. Therefore, the selection of brine injection pressure should be carefully and comprehensively considered regarding the factors of gas production and geological risks.
Conclusion
This study numerically verifies the feasibility of combined brine flooding with electrical heating–assisted depressurization in horizontal wells to improve gas production from the natural gas hydrate in the Shenhu area of the South China Sea. By analyzing the simulation results of methane recovery, water production, and energy gain, the optimizations of electrical heating time and power and brine injection pressure are achieved, and the following conclusions can be drawn:
Thermal stimulation by combined brine flooding with electrical heating can greatly improve methane recovery. After 20 years of production, the cumulative methane production of combined brine injection with electrical heating–assisted depressurization is 1.41 times of that conducted by the only depressurization method. However, the rather low energy efficiency ratio of the thermal stimulation method results in a similar net energy gain with the only depressurization method.
In order to improve energy efficiency, the advanced termination of electrical heating is proposed and numerically evaluated. The simulation results of three different termination times indicate that stopping electrical heating prematurely is disadvantageous to methane production due to insufficient hydrate dissociation. At the same time, keeping on electrical heating after 70% of hydrate dissociation results in massive energy wastes. Therefore, a medium electrical heating time is preferred for gas production from the hydrate deposit, whose superiority is proven by the largest net energy gain and a satisfactory energy efficiency ratio.
Increasing electrical heating power and brine injection pressure leads to better exploitation performance with higher methane recovery and net energy gain. However, the degree of improvement is gradually weakened after a certain threshold; in the meantime, the risks of wellbore and reservoir failures increase with these factors. Therefore, the selection of electrical heating power and injection pressure should be performed carefully and comprehensively, considering both the efficiency of the gas recovery and the risks of geological hazard.
This study only optimized the artificial operations of the tripartite exploitation strategy, however, the effect of reservoir physical property, hydrate saturation, and fluid component on the gas recovery has not yet been well-revealed and will be our next stage of investigation. In addition, comprehensive comparison with other electrical heating methods, for example, low-frequency electrical heating and electromagnetic heating, remains to be conducted.
Data Availability Statement
The raw data supporting the conclusion of this article will be made available by the authors, without undue reservation.
Author Contributions
QZ: conceptualization, methodology, data curation, visualization, and writing—original draft. YW: conceptualization, methodology, visualization, writing—review and editing, and supervision.
Funding
The research is supported by the Original Innovation Research Program of the Chinese Academy of Sciences (CAS) under Grant number ZDBS-LY-DQC003, and the Key Research Program of the Institute of Geology and Geophysics, CAS under Grant numbers IGGCAS-2019031 and SZJJ-201901.
Conflict of Interest
The authors declare that the research was conducted in the absence of any commercial or financial relationships that could be construed as a potential conflict of interest.
Publisher’s Note
All claims expressed in this article are solely those of the authors and do not necessarily represent those of their affiliated organizations, or those of the publisher, the editors, and the reviewers. Any product that may be evaluated in this article, or claim that may be made by its manufacturer, is not guaranteed or endorsed by the publisher.
Acknowledgments
We are grateful to editors and reviewers for important questions and suggestions.
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Keywords: natural gas hydrate, numerical simulations, brine injection, electrical heating, depressurization, Shenhu area
Citation: Zhang Q and Wang Y (2022) Numerical Simulations of Combined Brine Flooding With Electrical Heating–Assisted Depressurization for Exploitation of Natural Gas Hydrate in the Shenhu Area of the South China Sea. Front. Earth Sci. 10:843521. doi: 10.3389/feart.2022.843521
Received: 04 January 2022; Accepted: 07 February 2022;
Published: 02 March 2022.
Edited by:
Pibo Su, Guangzhou Marine Geological Survey, ChinaReviewed by:
Bo Li, Chongqing University, ChinaXianying Wang, Guangzhou Marine Geological Survey, China
Cheng Lu, China Geological Survey, China
Copyright © 2022 Zhang and Wang. This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
*Correspondence: Yanfei Wang, yfwang@mail.iggcas.ac.cn