Zijian Li ¹ Noah J. Planavsky ² Christopher Reinhard ^1*

• ¹ School of Earth and Atmospheric Sciences, College of Sciences, Georgia Institute of Technology, Atlanta, Georgia, United States
• ² Department of Earth and Planetary Sciences, Faculty of Arts and Sciences, Yale University, New Haven, Connecticut, United States

In an effort to mitigate anthropogenic climate impacts the U.S. has established ambitious Nationally Determined Contribution (NDC) targets, aiming to reduce greenhouse gas emissions by 50% before 2030 and achieving net-zero emissions by 2050. Enhanced rock weathering (ERW) -the artificial enhancement of chemical weathering of rocks to accelerate atmospheric CO2 capture -is now widely seen as a potentially promising carbon dioxide removal (CDR) strategy that could help to achieve U.S. climate goals. Grinding rocks to smaller particle size, which can help to facilitate more rapid and efficient CO2 removal, is the most energy-demanding and cost-intensive step in the ERW life cycle. As a result, accurate life cycle analysis of ERW requires regional constraints on the factors influencing the energetic and economic demands of feedstock grinding for ERW. Here, we perform a statelevel geospatial analysis to quantify how carbon footprints, costs, and energy demands vary among regions of the coterminous U.S. in relation to particle size and regional electricity mix. We find that CO2 emissions from the grinding process are regionally variable but relatively small compared to the CDR potential of ERW, with national averages ranging between ~5 -35 kgCO2 trock -1 for modal particle sizes between ~10 -100 µm. The energy cost for feedstock grinding also varies regionally but is relatively small, with national average costs for grinding of roughly 0.95 -5.81 $ trock -1 using grid mix power and 1.35-8.26 $ trock -1 (levelized) for solar PV for the same particle size range. Overall energy requirements for grinding are also modest, with the demand for grinding 1 Gt of feedstock representing less than 2% of annual national electricity supply. In addition, both cost and overall energy demand are projected to decline over time. These results suggest that incorporating feedstock grinding into ERW deployment at scale in the coterminous U.S. should generally have only modest impacts on lifecycle emissions, cost-effectiveness, and energy efficiency.